I think the title sums it up. The Harder They Come soundtrack is amazing. It has it all, The Slickers, Toots and the Maytals, Scotty, Desmond Dekker, and of course, Jimmy Cliff. another few that come to mind include, Trainspotting, The Royal Tenenbaums, and Ghost World. I also love The Life Aquatic Soundtrack. Bowie rules. Almost forgot about Natural Born Killers. <3 Patti Smith.